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Mohammadi, Abolfazl, Aryaeipanah, Mohammad, Hakimizadeh, Maryam. (1401). Dissociation Enthalpy of Methane/Carbon dioxide/Nitrogen and Tetra n-butylammonium Chloride Semiclathrate Hydrates Using the Clausius-Clapeyron Equation. , 56(1), 123-131. doi: 10.22059/jchpe.2022.335066.1373
Abolfazl Mohammadi; Mohammad Aryaeipanah; Maryam Hakimizadeh. "Dissociation Enthalpy of Methane/Carbon dioxide/Nitrogen and Tetra n-butylammonium Chloride Semiclathrate Hydrates Using the Clausius-Clapeyron Equation". , 56, 1, 1401, 123-131. doi: 10.22059/jchpe.2022.335066.1373
Mohammadi, Abolfazl, Aryaeipanah, Mohammad, Hakimizadeh, Maryam. (1401). 'Dissociation Enthalpy of Methane/Carbon dioxide/Nitrogen and Tetra n-butylammonium Chloride Semiclathrate Hydrates Using the Clausius-Clapeyron Equation', , 56(1), pp. 123-131. doi: 10.22059/jchpe.2022.335066.1373
Mohammadi, Abolfazl, Aryaeipanah, Mohammad, Hakimizadeh, Maryam. Dissociation Enthalpy of Methane/Carbon dioxide/Nitrogen and Tetra n-butylammonium Chloride Semiclathrate Hydrates Using the Clausius-Clapeyron Equation. , 1401; 56(1): 123-131. doi: 10.22059/jchpe.2022.335066.1373

Dissociation Enthalpy of Methane/Carbon dioxide/Nitrogen and Tetra n-butylammonium Chloride Semiclathrate Hydrates Using the Clausius-Clapeyron Equation

Journal of Chemical and Petroleum Engineering
دوره 56، شماره 1، شهریور 2022، صفحه 123-131    اصل مقاله (1.12 M)
نوع مقاله: Research Paper
شناسه دیجیتال (DOI): 10.22059/jchpe.2022.335066.1373
نویسندگان
Abolfazl Mohammadi* 1؛ Mohammad Aryaeipanah2؛ Maryam Hakimizadeh2
1Department of Chemical Engineering, University of Bojnord, Bojnord, Iran.
2Department of Chemical Engineering, University of Bojnord, Bojnord, Iran
چکیده
Due to high storage capacity, high dissociation enthalpy, and the appropriate melting point of gas hydrates, these compounds have a potential for many industrial applications. Tetra n-butylammonium halides are typical guest molecule involved in the formation of semiclathrate hydrates. In this manuscript, the dissociation enthalpy of methane/carbon dioxide/nitrogen + Tetra n-butylammonium Chloride semiclathrate hydrates is evaluated using the Clausius-Clapeyron equation. The equilibrium data are measured in a 460 cm3 stirred batch reactor using an isochoric pressure-search method. The dissociation enthalpy data were evaluated in the temperature range of (275.15 to 304.75) K and the pressure range of (0.36 to 10.57) MPa at (0 - 0.36) mass fraction of Tetra n-butylammonium Chloride. The results showed that the utilization of Tetra n-butylammonium Chloride increases the amount of dissociation enthalpy of semiclathrate hydrates per mole of the hydrated gas. By increasing the mass fraction of Tetra n-butylammonium Chloride, the amount of dissociation enthalpy per mole of hydrated gas increased.
کلیدواژه‌ها
Clausius-Clapeyron؛ Dissociation Enthalpy؛ Gas Hydrates؛ Semiclathrates؛ Tetra-n-Butylammonium Chloride
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آمار
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