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Highly Adsorption-Photocatalytic Tablet-Shaped Graphite Oxide-TiO2 Composites for Handling Organic Dye Pollutants | ||
| Journal of Chemical and Petroleum Engineering | ||
| دوره 58، شماره 2، اسفند 2024، صفحه 277-288 اصل مقاله (642.09 K) | ||
| نوع مقاله: Research Paper | ||
| شناسه دیجیتال (DOI): 10.22059/jchpe.2024.370403.1475 | ||
| نویسندگان | ||
| Dwiprayogo Wibowo* 1؛ Faizal Mustapa2؛ Albi Fabian3؛ Eza Rezki Fitaloka4؛ Dedi Ardiansyah5؛ Aryani Adami6؛ Anwar Said7؛ Jamal Mukaddas6؛ Abriansyah Abriansyah7 | ||
| 1Jl. KH. Ahmad Dahlan. | ||
| 2Department of Marine Sciences, Institute of Teknologi dan Bisnis Muhammadiyah Kolaka | ||
| 3Department of Environmental Engineering, Faculty of Engineering, Muhammadiyah University of Kendari. | ||
| 4Department of Medical and Electrical Engineering, Faculty of Science and Technology, University of Mandala Waluya. | ||
| 5Fishery Products Technology, Faculty of Fisheries and Marine Science, Muhammadiyah University of Kendari. | ||
| 6Department of Urban and Regional Planning, Faculty of Engineering, Lakidende University. | ||
| 7Department of Mining Engineering, Faculty of Engineering, Muhammadiyah University of Kendari. | ||
| چکیده | ||
| Designing effective adsorption-photocatalysts on graphite oxide-TiO2 (G/TiO2) nanocomposites tablet with easy synthesis and low cost is a challenge in treating organic dye pollutants. Here, we invented an advanced adsorption-photocatalyst based on a TiO2 framework coupled with graphite oxide to form tablets using a physical mixing method. Furthermore, these tablets were molded using metal chips for extremely high adsorption photocatalysts towards organic dyes. The mass composition has been evaluated to compare the high degradation performance of the composite mass variation in degrading organic dyes, namely methyl orange (MO) and methylene blue (MB). We discovered the 1:2 mass variation of G/TiO2 resulted in an improvement in the adsorption-photocatalytic degradation of organic dyes. The degradation rate of MO dye was 93.99% after treatment with UV light irradiation for 60 min, and the reaction rate constant was k = 0.01726 min-1. Meanwhile, MB dye also showed good performance with a degradation percentage of 80.22% and a reaction rate constant of k = 0.00947 min-1. This constant was much higher than the two mass variations (1:1 and 2:1) of G/TiO2 due to the increased availability of good sites for graphite oxide adsorption and TiO2 electron-hole pair separation. In addition, the G/TiO2 tablets showed excellent reuse and reasonable degradation for wastewater treatment. | ||
| کلیدواژهها | ||
| Adsorption؛ Graphite؛ Organic Dyes؛ Photocatalyst؛ TiO2 | ||
| مراجع | ||
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