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کاربرد معادلات سینتیکی در توصیف سرعت آزاد شدن سرب در یک خاک آهکی تیمارشده با بیوچارهای مختلف | ||
| تحقیقات آب و خاک ایران | ||
| دوره 55، شماره 5، مرداد 1403، صفحه 815-832 اصل مقاله (1.87 M) | ||
| نوع مقاله: مقاله پژوهشی | ||
| شناسه دیجیتال (DOI): 10.22059/ijswr.2024.370481.669639 | ||
| نویسندگان | ||
| پروین کبیری1؛ علیرضا حسین پور1؛ حمیدرضا متقیان* 1؛ رامین ایرانی پور2 | ||
| 1گروه علوم خاک، دانشکده کشاورزی، دانشگاه شهرکرد، شهرکرد، ایران. | ||
| 2واحد آب و خاک، سازمان ﺗﺤﻘﯿﻘﺎت، آموزش و ترویج ﮐﺸﺎورزی، شهرکرد، ایران. | ||
| چکیده | ||
| فعالیت‌های معدن‌کاوی، موجب ورود و تجمع فلزات سنگین در خاک می‌شود. بیوچار، می‌تواند چنین خاک‌های آلوده‌ای را پاک‌سازی کند. در این پژوهش تأثیر کاربرد 2 درصد وزنی/وزنی بیوچارهای تهیه‌شده (در دمای 600 درجه سلسیوس) از بقایای مختلف بر قابلیت استفاده و سرعت آزادشدن سرب در خاک آلوده معدن بررسی شد. خاک آهکی لوم‌شنی که از نزدیکی معدن سرب و روی باما واقع در شهر سپاهان شهر نمونه‌برداری شد، با بقایا و بیوچارهای تهیه‌شده از آنها به‌مدت 120 روز خوابانده و سپس مقدار قابل استفاده و سرعت آزادشدن سرب در خاک شاهد و تیمارها پس از عصاره‌گیری با محلول دی‌اتیلن‌تری‌آمین‌پنتا استیک اسید (DTPA-TEA) در طول مدت 504 ساعت اندازه‌گیری گردید. نتایج نشان داد که پس از تیمار خاک با بیوچارها، سرب قابل استفاده و سرعت آزادشدن سرب در تیمارها نسبت به شاهد به طور معنی‌داری کاهش یافت. مقایسه ضریب تبیین (R2) و خطای استاندارد برآورد (SEE) نشان داد که معادله‌های الوویچ ساده، تابع توانی و مرتبه اول دارای بیشترین ضریب تبیین و کمترین خطای استاندارد برآورد برای خاک‌های شاهد و تیمارشده بوده و بنابراین توانایی توصیف سرعت آزادشدن سرب را در این خاک‌‌ها داشتند. ضریب 1/β در معادله الوویچ و b در معادله تابع توانی به‌ترتیب در دامنه 47/161 – 18/237 میلی‌گرم بر کیلوگرم بر ساعت و 245/0 – 299/0 میلی‌گرم بر کیلوگرم بر ساعت به دست آمد. نتایج مطالعات همبستگی بین سرب عصاره‌گیری شده با DTPA-TEA و ضرایب معادلات در این پژوهش، نشان داد که ضرایب K1، 1/β، b و a*b برای توصیف سرعت آزادشدن سرب مفیدتر و به واقعیت نزدیک‌تر بودند. | ||
| کلیدواژه‌ها | ||
| کمپوست زباله شهری؛ لجن فاضلاب شهری؛ بقایای گیاهی؛ بقایای باغی | ||
| عنوان مقاله [English] | ||
| Modeling the kinetic equations in describing the release rate of lead in a naturally contaminated calcareous soil treated with different biochars | ||
| نویسندگان [English] | ||
| parvin kabiri1؛ alireza hosseinpur1؛ Hamidreza Motaghian1؛ ramin iranipour2 | ||
| 1Department of Soil Science, Faculty of Agriculture, Shahr-e-kord University, Shahr-e-kord, Iran. | ||
| 2water and soil unit, agricultural research, education and extension organization,, Shahr-e-kord, Iran. | ||
| چکیده [English] | ||
| Mining activities provide a pathway for the entry and accumulation of heavy metals in soil. Utilization of biochars could remediate such contaminated soils. Therefore, in this study, the impact two percent of different wastes and biochars (prepared at temperature of 600 °C) was investigated on the availability and release kinetics of lead in polluted soil. Sandy loam calcareous soil, which was collected near Bama lead and zinc mine located in Sepahan Shahr city, was treated with residues and biochars and incubated for 120 days. Then the availability and release kinetics of lead were measured in control and treatments extracting with diethylenetriaminepentaacetic acid solutions (DTPA-TEA) during 504 hours. Results showed that treating soils with biochars, decreased the bioavailablaty and release kinetics of Pb significantly in comparison with control. The comparison of the coefficient of explanation (R2) and the standard error of estimation (SEE) of equations showed that simple Elovich equations, power function and first order equations had the highest coefficient of explanation and the lowest standard error of estimate for control and treated soils. So, these mathematical equations have been useful in explaining the cumulative release and release rate of Pb. Values of 1/β (derived from the simplified Elovich equation) and b (derived from the power function equation) changed from 161.47 – 237.18 mg kg-1 h-1 and 0.245 – 0.299 mg kg-1 h-1, respectively. Correlation analysis study, between DTPA-Pb with constants illustrated that among the constants, “K1”, “1/β”, “b”, and “a*b” were better parameters to predict the release kinetics of Pb. | ||
| کلیدواژه‌ها [English] | ||
| urban waste compost, sewage sludge, waste crops, waste products | ||
| مراجع | ||
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